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Bloom, Rev. Pure Appl. Chem. 7:389 (1963). 26. G. J. Janz, R. D. Reeves, and A. T. Ward, Nature 204:1188 (1964). 27. J. E. , H. A. A. Abdel-Rehim, and S. W. Rudich, J. Phys. Chem. 70:3610 (1966). 28. C. A. Angell and C. T. Moynihan, in: Molten Salts, Characterization and Analysis (G. ), pp. 315-375, Marcel Dekker, New York (1969). 29. A. J. Easteal and C. A. Angell, Aust. J. Chem. 23:929 (1970). 30. R. W. Laity, J. Chem. Phys. 30:682 (1959). 31. G. Morrison and J. E. , J. Phys. Chem. 72:3001 (1968).
2) According to the authors, if the gas does not interact with liquid, the free energy change upon mixing is related to the surface energy of the "hole" created by the gas. The cavities are considered to be of molecular or atomic size and the surface tension of the solvent along the walls of the cavity is taken to be equal to the macroscopic value. In spite of the many assumptions, the equations appear to predict the observed solubilities. The solubility relationship given by these authors is (1) where Cg is the concentration of gas in the gas phase in equilibrium with the gas in the liquid at a concentration Cd, and A is the total surface area of the spherical cavity.
T. Ward, Nature 204:1188 (1964). 27. J. E. , H. A. A. Abdel-Rehim, and S. W. Rudich, J. Phys. Chem. 70:3610 (1966). 28. C. A. Angell and C. T. Moynihan, in: Molten Salts, Characterization and Analysis (G. ), pp. 315-375, Marcel Dekker, New York (1969). 29. A. J. Easteal and C. A. Angell, Aust. J. Chem. 23:929 (1970). 30. R. W. Laity, J. Chem. Phys. 30:682 (1959). 31. G. Morrison and J. E. , J. Phys. Chem. 72:3001 (1968). 32. E. Helfand, Phys. Fluids 4:681 (1961). 33. H. C. Longuet-Higgins and J.